OPTIMIZATION SEMINAR



Geometry Optimizations in Quantum Chemistry




Mark S. Gordon
Professor of Chemistry
Iowa State University

Tuesday, Sep. 9, 1997, 12:00 noon
CU-Denver Bldg., Room 626


Abstract

The central issues in the application of quantum mechanics to solving problems in chemistry are determination of molecular structures and related properites (e.g., vibrational frequencies, electric and magnetic moments, NMR and ESR properties), elucidation of the nature of chemical bonding, and the determination of reaction mechanisms in the gas and condensed phases. All of these problems require careful determination of molecular geometries, not only at local minima, but also at saddle points connecting relevant minima and at large numbers of points along reaction paths and reaction trajectories. These problems require increasingly sophisticated optimization algorithms as the size of the systems increases, and is especially exacerbated in liquid and solid systems. After an introduction to electronic structure theory and our quantum chemistry program GAMESS, several problems of increasing complexity will be discussed.